To propose a guideline for membrane design, a process simulation was conducted for conversion enhancement as a function of pressure difference using Aspen HYSYS ®. The SMR test was conducted at 823 K with a steam-to-carbon ratio of 3.0 and gas hourly space velocity of 1000 h −1 increasing the pressure difference resulted in enhanced methane conversion, which reached 82% at a pressure difference of 912 kPa. The Pd-based composite membrane had a hydrogen permeance of 2.4 × 10 −3 mol m −1 s −1 Pa −0.5 and an H 2/N 2 selectivity of 618 at a temperature of 823 K and a pressure difference of 10.1 kPa. A Pd-based composite membrane with a thickness of 4–5 μm was prepared on a tubular stainless steel support (diameter of 12.7 mm, length of 450 mm) using electroless plating (ELP).
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